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Process Optimization and Techno-Economic Assessment of CO2 Capture Using a Polymeric Solvent System

高分子溶媒システムを用いたCO2回収のプロセス最適化と技術経済評価 (AI 翻訳)

Yousuf Bin Arif, Abu Hurairah Hassnain, Nouman Harris, S. Haq, Saad Nadeem, S. M. Lalji, Syed Imran Ali

Offshore Technology Conference学会2026-04-27#CCUSOrigin: Global
DOI: 10.4043/37034-ms
原典: https://doi.org/10.4043/37034-ms

🤖 gxceed AI 要約

日本語

本研究は、水溶性ポリマー溶媒であるカルボキシメチルスターチナトリウム(Na-CMS)を用いたCO2回収プロセスの最適化と技術経済評価を実施。Aspen Plusを用いた定常状態モデルにより、吸収塔温度30°C、圧力10 bar、溶媒循環量26 kmol/hの条件下で98%のCO2回収効率を達成。感度分析では、エネルギー負荷、回収率、炭素価格が経済性に最も影響することが示された。Na-CMSは更なる材料改良により商業化の可能性がある。

English

This study investigates sodium carboxymethyl starch (Na-CMS) as a polymeric solvent for post-combustion CO2 capture, using Aspen Plus simulation and techno-economic assessment. Optimal performance at 30°C, 10 bar, and 26 kmol/h solvent circulation achieved 98% CO2 capture efficiency. Sensitivity analysis highlights energy duty, capture rate, and carbon price as key economic drivers. Na-CMS shows promise as a tunable platform for carbon capture, though experimental validation is needed.

Unofficial AI-generated summary based on the public title and abstract. Not an official translation.

📝 gxceed 編集解説 — Why this matters

日本のGX文脈において

CCUSは日本のGX政策において重要な位置を占めており、特に既存火力発電所や産業プロセスへの適用が期待される。本研究成果は、低コストで効率的なCO2回収技術の開発に寄与し、日本の排出削減目標達成に向けた技術選択肢を拡充する。

In the global GX context

This paper contributes to the global CCUS literature by evaluating a novel polymeric solvent system with high capture efficiency and economic viability. The techno-economic framework and sensitivity analysis provide practical insights for scaling up carbon capture technologies, relevant for industrial decarbonization efforts worldwide.

👥 読者別の含意

🔬研究者:Provides a simulation-based assessment of Na-CMS for CO2 capture, offering a baseline for further material and process optimization.

🏢実務担当者:Presents an economic evaluation of a novel solvent system, useful for companies considering CCUS technology investments.

🏛政策担当者:Highlights the importance of carbon pricing and energy costs in CCUS economics, informing policy design for carbon capture incentives.

📄 Abstract(原文)

Post-combustion carbon capture remains an essential option for reducing industrial greenhouse gas emissions; however, conventional solvent systems continue to face limitations related to operational stability and environmental sustainability. This study examines sodium carboxymethyl starch (Na-CMS), a water-soluble polymeric solvent, as a non-reactive platform for CO2 capture and process optimization. Despite growing interest in polymer-based absorbents, their performance in absorber-stripper configurations under realistic operating conditions remains insufficiently understood. To address this gap, a steady-state absorber-regeneration configuration was developed in Aspen Plus to evaluate CO2 absorption using Na-CMS in a tray column system. Key process and economic parameters were evaluated through a scenario-based techno-economic framework, with system performance assessed using Net Present Value (NPV), Levelized Cost of Carbon Capture (LCOCC), Return on Investment (ROI), and Payback Period (PBP). Three representative cases were analyzed to identify economic thresholds and feasibility limits. An overall CO2 capture efficiency of 98% was attained with Na-CMS. The optimized operating region was identified at an absorber temperature of 30 °C, a moderate operating pressure of 10 bars, and a solvent circulation rate of 26 kmol.h-1. Under these conditions, simulated CO2 removal exceeded typical polymeric-solvent efficiency and delivered predictable trade-offs between capture fraction and energy penalty. Sensitivity analysis showed that energy duty, capture rate, and carbon price most strongly influence project economics. Na-CMS emerges as a tunable platform for further materials and process refinement; experimental validation and targeted material modification are recommended to reduce regeneration duty and improve commercial prospects.

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