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A Durable Membrane-Free Platform for Green Hydrogen and High-Purity Ammonium Recovery Powered by Human Urine Remediation

尿処理を動力源とするグリーン水素と高純度アンモニウム回収のための耐久性のある膜フリープラットフォーム (AI 翻訳)

Jang A, Nguyen DA, Thi KAN, Kim T, Im H

Research Squareプレプリント2026-08-05#水素経営インパクト: コスト削減対象セクター: wastewater_treatment
DOI: 10.21203/rs.3.rs-10574110/v1
原典: https://doi.org/10.21203/rs.3.rs-10574110/v1

🤖 gxceed AI 要約

日本語

ヒト尿から高純度アンモニウムを回収しつつ、水素を同時生産する膜フリープラットフォームを開発。固定化ウレアーゼビーズとKCoHCF電極により、尿素の98%以上を加水分解し、アンモニウムを99.9%の選択性で回収。有機物の82%を除去し、正味エネルギー利得(-0.47 kWh/kg-N)を達成。物理情報に基づく劣化モデルでシステム寿命を高精度に予測し、自律運用を可能にする。

English

This platform recovers high-purity ammonium from human urine while co-producing hydrogen, powered by its own organics. It achieves >98% urea hydrolysis, ~90% ammonium capture with 99.9% selectivity, and 82% organic removal, with a net energy gain (-0.47 kWh/kg-N). A physics-informed degradation model predicts system lifetime accurately, enabling autonomous operation.

Unofficial AI-generated summary based on the public title and abstract. Not an official translation.

📝 gxceed 編集解説 — Why this matters

日本のGX文脈において

日本では下水道の維持管理コストや窒素負荷が課題であり、本技術は尿由来の資源回収と水素製造を両立する点で、循環型社会や水素社会の実現に寄与する。特に、地域分散型のエネルギー・資源循環システムとして、自治体や企業の脱炭素施策に応用が期待される。

In the global GX context

Globally, this work addresses the energy-intensive nitrogen cycle by turning urine from a waste into a resource, aligning with circular economy and green hydrogen goals. It offers a decentralized solution for nutrient recovery and renewable energy production, relevant to sustainable sanitation and hydrogen economy strategies.

👥 読者別の含意

🔬研究者:Provides a novel membrane-free approach for simultaneous ammonium recovery and hydrogen production, with a physics-informed degradation model for system longevity.

🏢実務担当者:Offers a potential decentralized solution for wastewater treatment plants to recover valuable nutrients and produce green hydrogen, reducing operational costs.

🏛政策担当者:Highlights a technology that can support circular economy policies and renewable hydrogen targets, particularly for decentralized sanitation and resource recovery.

📄 Abstract(原文)

<title>Abstract</title> <p> Conventional sanitation runs a self‑defeating loop: energy is spent destroying nitrogen in wastewater while industry expends more to fix it anew from air. Human urine carries most of that nitrogen, and here we turn this disposal cost into a resource. Our durable, membrane‑free platform recovers high‑purity ammonium from raw, undiluted urine and co‑produces hydrogen, powered by its own organics. Immobilized urease beads hydrolyze >98% of urea, and a record-surface-area KCoHCF electrode selectively captures ~90% of ammonium at 99.9% selectivity and a recovery rate of ~1,100 g-N.m <sup>-2</sup> .d <sup>-1</sup> , rejecting Na <sup>+</sup> by 2,300-fold and K <sup>+</sup> by 10-fold while retaining 93% capacity over 1,000 cycles through breathing effect. The platform simultaneously removes 82% of organic matter and operates with a net energy gain (−0.47 kWh kg <sup>-1</sup> -N), enabling profitable operation at medium- and large-campus scales. A physics-informed degradation model accurately predicts system lifetime without large training datasets, outperforming existing approaches and enabling autonomous long-term operation. </p>

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