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Cross‐Scale Coupling Perspective: A New Pathway to Break the Selectivity Dilemma of Electrocatalytic Energy Conversion Reactions

クロススケール結合の視点:電解触媒エネルギー変換反応の選択性ジレンマを打破する新経路 (AI 翻訳)

Zilong Chen, Yaxuan Huang, Zihan Wang, Suping Li, Guohui Qin, Lei Wang, Jianping Lai

Chemistry - A European Journal📚 査読済 / ジャーナル2026-08-14#エネルギー転換Origin: CN
DOI: 10.1002/chem.71576
原典: https://doi.org/10.1002/chem.71576

🤖 gxceed AI 要約

日本語

本レビューは、電解触媒の選択性制御におけるナノからマクロまでのクロススケール統合の重要性を論じ、既存研究の単一スケール偏重を批判する。産業応用に向けた理論的枠組みを提案し、AI統合による触媒設計の将来展望を示す。

English

This review argues for cross-scale integration in electrocatalytic selectivity, from nano to macro, criticizing single-scale approaches. It proposes a theoretical framework for industrial application and highlights AI integration for future catalyst design.

Unofficial AI-generated summary based on the public title and abstract. Not an official translation.

📝 gxceed 編集解説 — Why this matters

日本のGX文脈において

日本の水素社会実現やカーボンニュートラル政策において、グリーン水素製造の効率向上に寄与する可能性がある。ただし、具体的な産業応用にはまだ距離があり、基礎研究段階の知見として位置づけられる。

In the global GX context

This paper contributes to global efforts in green hydrogen and CO2 conversion, aligning with decarbonization pathways. It underscores the need for cross-scale thinking to bridge lab-to-industry gaps, relevant for clean energy technology development.

👥 読者別の含意

🔬研究者:電解触媒の選択性制御におけるクロススケール研究の方向性を示す。

📄 Abstract(原文)

Against the backdrop of global energy transition and carbon neutrality goals, electrocatalysis stands as a core technology for efficient conversion of renewable energy and green chemical synthesis, and its selectivity regulation has become a prominent research hotspot. Nevertheless, most existing studies focus merely on a single scale, such as atomic-level electronic structures or macroscopic mass transfer, while neglecting cross-scale synergistic regulation spanning from nanoactive sites to mesoscopic interfaces and further to macroscopic reactors. This renders the selectivity performance achieved under ideal laboratory conditions difficult to meet the complex dynamic requirements of industrial high-current-density and supported catalyst systems, giving rise to a distinct gap between fundamental research and industrial practical applications. This paper systematically reviews the regulation of electrocatalytic selectivity, aiming to construct a comprehensive theoretical framework for cross-scale selectivity regulation across macroscale, mesoscale, and nanoscale with full-scale coverage and in-depth elaboration. The research scope covers multiple levels, including active sites, interfacial environments, and external field responses. Future research should prioritize deepening the integration of artificial intelligence and electrocatalysis to enable intelligent catalyst design, develop self-adaptive catalyst systems to optimize dynamic reaction processes, and accelerate industrial applications in green hydrogen production, carbon dioxide conversion, and other related fields.

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